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Cours de chimie des lanthanides

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Les lanthanides – 1. Découverte et propriétés fondamentales
Claude Piguet (Genève)

17 février 2009

Bibliographie :
• Johnson, D.A. Some Thermodynamic Aspects of Inorganic Chemistry, 2nd ed., Cambridge University Press, Cambridge, 1982.
• Kaltsoyannis N., Scott P. The f Elements, Oxford Science Publication, Oxford, 1999.
• Saez-Puche R., Caro P., eds. Rare Earthes, Editorial Complutense SA, Madrid, 1998.
• Sastri V.S., Bünzli J.-C.G., Rao V.R., Rayudu G.V.S., Perumareddi J.R. Modern Aspects of Rare Earths and Their Complexes, Elsevier, Amsterdam, 2003.
• Choppin G.R. In Lanthanide Probes in Life, Chemical and Earth Sciences, Bünzli J.-C.G., Choppin G.R., eds., Elsevier, Amsterdam 1989, chap. 1.
• Cotton S. Lanthanide and Actinide Chemistry, John Wiley & Sons Ltd, Chichester, 2006.

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Non disponible Claude Piguet (Genève)
Claude Piguet earned a Ph.D. degree in 1989 from the University of Geneva in the field of biomimetic copper-dioxygen complexes. After several postdoctoral periods (on supramolecular chemistry, coordination chemistry, and photophysics of rare earths), he initiated research projects in the field of the lanthanide supramolecular chemistry. In 1995 he received the Werner Medal of the New Swiss Chemical Society and the Werner fellowship from the Consortium of the Swiss Chemical Industries. He was appointed in 1999 as full professor of inorganic chemistry and occupies the chair of f-element of the University of Geneva. He coauthored more than 150 scientific articles and book chapters in various fields of chemistry, which include the design of discrete multimetallic supramolecular edifices and the unravelling of the thermodynamic origin of their self-assembly processes, the programming of novel electronic functions depending on intermetallic communications, the molecular tuning of apparent local dielectric constants, the microscopic rationalization of phase transitions, the preparation of lanthanide-containing metallomesogens and the development of paramagnetic NMR methods for addressing solution structures.
Selected key publications :
• Dalla Favera N., Hamacek J., Borkovec M., Jeannerat D., Gumy F., Bünzli J.-C.G., Ercolani G., Piguet C. "Linear polynuclear helicates as a link between discrete supramolecular complexes and programmed infinitie polymetallic chains", Chem. Eur. J. 14 (2008), 2994–3005.
• Canard G., Koeller S., Bernardinelli G., Piguet C. "Effective concentration as a tool for quantitatively addressing preorganization in multicomponent assemblies: application to the selective complexation of lanthanide cations", J. Am. Chem. Soc. 130 (2008), 1025–1040.
• Piguet C., Bünzli J.-C.G., Donnio B., Guillon D. "Thermotropic lanthanidomesogens", Chem. Commun. (2006), 3755–3768.
• Hamacek J., Borkovec M., Piguet C. "Simple thermodynamics for unravelling sophisticated self-assembly processes", Dalton Trans. (2006), 1473–1490.
• Piguet C., Geraldes C.F.G.C. "Paramagnetic NMR lanthanide induced shifts for extracting solution structures", in Handbook on the Physics and Chemistry of Rare Earths, Gschneidner Jr. K.A., Bünzli J.-C.G., Pecharsky V.K. eds., Elsevier Science, Amsterdam, 33 (2003), 353–463.
• Bünzli J.-C.G., Piguet C. "Lanthanide-containing molecular and supramolecular polymetallic functional assemblies", Chem. Rev. 102 (2002), 1897–1928.

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